Published: Aug. 27, 2019

New technique from CU 麻豆影院 researchers could free quantum technology from cold temperatures


Research on quantum states of matter could be conducted at room temperatures, thus facilitating cheaper and more widely available quantum technologies, research at the 麻豆影院 suggests.

May

Graduate student Molly May aligns optics in the scanning probe apparatus that controls the quantum dot emission. Photo courtesy of Molly May. At the top of the page is an artist's illustration of听tip-enhanced strong coupling for room temperature quantum technologies.听Credit: Steven Burrows/JILA.

鈥淭his is exploratory research on quantum emitter put into novel very tiny optical nano-cavities. It allows for controlling quantum states even at room temperature which can create a wider range of quantum platforms and broader accessibility,鈥 said Markus Raschke, CU 麻豆影院 professor of physics and JILA fellow.听

鈥淲e are extending the application space of quantum technologies into more real world applications, operating even under ambient conditions, from sensing to new chemistry, which is really exciting,鈥

鈥淭ypically, quantum physics and tailored light-matter interactions requires ultracold, ultrahigh vacuum, very pristine conditions,鈥 added Molly May, a JILA graduate student in the Raschke group, who explained why room-temperature quantum state control is important:听

鈥淚f we want to use these technologies more broadly, it's so much cheaper, and would find so much wider use, if we were able to do it in your lab or your office or even your living room.鈥澨

Results of the research, which was done in collaboration with researchers at the University of Maryland, were published recently in the journal Science Advances.

Quantum research in ultracold conditions鈥攏ear absolute zero鈥攊s important as quantum technologies are probed and developed.听

But Earth is a warm place. 鈥淲e live in a heat bath,鈥 May joked, expounding on the basics of quantum research:听

Despite their small size, atoms have the ability to carry and transfer information, which makes them a听promising platform for quantum sensing, metrology and information processing.听

However, artificial atoms in the form of 鈥渜uantum dots" can also encode such information, andthe information in those quantum dots can equally be controlled with light, May explained.

But quantum dots and atoms tend to lose the information rapidly to their surroundings, so one has to operate on them quickly and precisely. That typically means working in extremely cold temperatures.听Extremely cold temperatures 鈥渇reeze鈥 the atoms, reducing their interaction with their environment鈥攚hich makes them easier to work with and control.听

But if controlling and working with atoms is restricted to cold temperatures, that would make it harder to take advantage of their quantum properties for wider range of applications outside of very specialized labs, added Raschke.

Writing on a nanoscale

The Raschke group works with quantum dots that are about 8 nanometers across, more than 1,000 times smaller than a human hair, but still much bigger compared to atoms.听

Raschke

Markus Raschke,听physics professor and JILA fellow, project principal investigator.

Writing information on a quantum dot involves changing its energy level from its ground state to an excited state. And photons鈥攖iny packets of energy that make up light鈥攃an do that when they strongly interact or couple with the quantum state.

When we saw the first data, they were almost too good to听be true.听We almost did not believe the results and thought something had gone wrong, some artifact, something is fooling us.鈥

But compared to the size of the quantum dots or atoms, visible light has a very long wavelength, almost a hundred times larger than the quantum dot. As a result, it has a very weak interaction with the quantum dot.听

The other problem is, that over time, the movement and coupling of an atom or quantum dot knocks its excitation out of phase with the light field. That phase decoherence causes the atom to lose its information to the surrounding environment.

There are two ways to work around this. One option is to work in high vacuum and at ultra-cold temperatures, usually around a few micro-Kelvin, to reduce the chances of this phase decoherence.听听

The new approach, as pursued by the Raschke group, is to squeeze the light into a very small space, much smaller than its wavelength, in fact comparable to the size of the quantum dot. Using nanoscale optical antennas made by metallic nanostructures, you can create such an optical nano-cavity, squeezing the light into exceedingly small dimensions. Then almost magically, the coupling becomes strong and fast, faster than the loss of the information you try to write, May explained.听

But those cavities are static. You either hit the quantum dot or you don鈥檛, May explained. 鈥淓ven when you get lucky and find a quantum dot, you cannot tune the cavity or control the interaction,鈥 she added.

Some like it hot

To work at room temperature and control the quantum state, May looked at an optical scanning probe technique, a technique already used at JILA that uses needle-like gold tip, as a tool to compress, or nano-focus, the light into the tiny space of only 10 nanometer in size at the tip of the needle, and as needed to get strong interaction with the quantum dot.听

When she shines light onto the gold tip, it focuses it into that nsmall region at the tip apex, creating an optical nanocavity with the quantum dot sample positioned between the tip and a flat gold mirror.

鈥淚t works like the antenna in your phone, just for light. The tip nano-cavity collects the light that we shine on it and focuses it to a tiny spot,鈥 May said.

The scanning probe microscope now provides the advantage that the tip can move around. So May can position the tip near the quantum dot with atomic precision. And when strong coupling sets in at very short distances between the tip and the quantum dot, the tip and the dot exchange information really well, tossing photons back and forth like ping-pong, May explained.听

鈥淎s we come closer and closer to the quantum dot, we see that the coupling kind of kicks in,鈥 May said. 鈥淚 was actually impressed by how well it works. And, that really hasn't been done before. We can really optimize, control, and image the interaction.鈥澨

Raschke was surprised by the results. 鈥淲hen you do a new experiment in science, you don鈥檛 want to put your hopes too high that it would actually work as you envision, to limit your disappointment when it doesn鈥檛. But when we saw the first data, they were almost too good to听be true.听We almost did not believe the results and thought something had gone wrong, some artifact, something is fooling us,鈥 he said. 鈥淚t was truly exhilarating when we saw the signal for the first time and gradually convinced ourselves it is real.鈥

Static cavities are like a picture鈥攜ou may get some interaction but you can鈥檛 turn a knob to control it, making it of very limited utility. Now it is like in a movie.听That strong-coupling effect using the tip lets May and her fellow researchers tune, control, and image the interaction with the quantum dot in real time and space. Pull the tip back, by a distance of even just one atom diameter, and the signal gets weaker. Push it closer, and the signal gets stronger.

Free from the fridge

Being able to write and read the energy level of a single quantum dot or atom using light is an enabling step for several emerging quantum technologies, like metrology and sensing tools. And breaking out of the ultra-cold regimes could help bring these tools out of the lab for wider applications, the team said.听

The new method of cavity nano-optics won鈥檛 get rid of the need for research and technologies at low temperature because of other important virtues, Raschke clarified. But this finding expands quantum science and technology into new regimes at room temperature with complementary benefits.听It also serves as a new tool to provide fundamental insight into how quantum information is lost in interacting environments, which can help optimize quantum systems more broadly.听

Their paper was published in Science Advances on July 12.听